There is no relationship between CR and stoichiometric fuel ratios. The increased flame front velocity from a higher compression ratio will somewhat affect the overall scavenge/breathing for a given physical configuration and valve (cam) spec. If anything, the ideal in a Model A going from 4.22 to 5.5 may require a slightly leaner mix, not richer.
You probably won't need to change anything if your car runs with properly colored plugs now. The nice thing about an A is you have a GAV to fiddle with a bit. If that doesn't find the sweet spot only then play with jet flow rates.