John,
Cranking cylinder pressure is not really relative to C/R.
So many factors combine to the cranking pressure that it is only a comparison from cyl to cyl.
Adding compression, or increasing the C/R is going to add performance.
At some point, the increase can be detrimental, ask around here, but be honest.
The condition of the base motor and the intended use are instrumental to success.
If the rings are worn, bearings/Babbitt is questionable then adding compression is just likely to finish off the motor sooner.
John