The compression ratio is the ratio of the volume of the combustion chamber (a), plus the volume of the cylinder (b), divided by the volume of the combustion chamber (a).
Or, (a + b)/a. This reduces to 1 + b/a.
If the original combustion ratio is 4.22, then 1 + b/a = 4.22, so b/a = 3.22.
Snyder's 6:1 head is listed to have a quench volume of 152 cc.
Your cylinder's are overbored 0.060". That increases the sweep volume (displacement) from 50.1 cu. in. to 51.69 cu.in. or 821 cc to 847 cc.
Assuming your gasket space volume is the same or the piston rises above the gasket, pop-up, this should not change. And, if your piston is flat (stock), no dome, then the quench volume stays the same.
Therefore, 0.060" over bore increases volume by about 1.5%. This changes the sweep volume (displacement) 3%.
displacement volume = pi x radius x radius x stroke length (4 1/4" in Henry's engine)
The 6.1 head decreases the combustion chamber by 41% but it is a much smaller volume than the cylinder volume.
so the calculation works out that your predicted CR should be 6.57:1 for an overbored engine by 0.060", stock piston with stock piston-pop-up, stock crank and rods, standard headgasket and appropriate torqued head nuts, standard valves (if your rebuilt valves ride high, they will consume some of the combustion chamber volume and the quench volume, subsequently the CR will go up because the combustion chamber is smaller), and standard plugs (the plugs take up some of the volume too by riding below the head.
The smaller plugs with the adapter increases the combustion chamber volume).
All these can affect the size of the combustion chamber the pistons are compressing the increased displacement volume into.
All the HC heads I have measured have CRs higher than stated, even in sleeved cylinders (returned to stock dimensions).
The Snyder's 6.1:1 head calculates to a 6.4:1 compression ratio if Henry, himself, were to place it on a new engine at the Rouge Plant.
I hope this helps.